Keeping it to things I think are slightly (emphasis on slightly) realistic, I'd most like Funi to license:
Strike Witches movie
Qwaser of Stigmata
Binbou Shimai Monogatari
Children who Chase Lost Voices from Deep Below
Although I reckon some of these might be more Sentai territory.
2. Eve no Jikan ONA (Time of EVE) also needs a blu ray release
This series is also highly rated, has beautiful artwork and a thought provoking insightful story.
The Japanese BD of the OVA already has English subtitles. For me, that's as good as licensed. Although I'd still double dip if an R1 company re-released it.